Barton Hollow

If you haven't checked out The Civil Wars then it's about time you did. Their music is so simple, pure, lovely, and yet powerful. It's really moving stuff.
I listened to their album, Barton Hollow, today and it's quite clear that these two have a beautiful musical chemistry. It's considered indie folk and has a slight country feel to it that isn't dripping with twang and my-girl-left-me-and-took-my-dog-and-my-truck-and-my-gun lyrics. This makes it anti-country listener friendly.
I highly suggest you check these two out.